Strong angular and spectral narrowing of electroluminescence in an integrated Tamm-plasmon-driven halide perovskite LED

Zher Ying Ooi, Alberto Jiménez-Solano,Krzysztof Gałkowski,Yuqi Sun,Jordi Ferrer Orri,Kyle Frohna,Hayden Salway,Simon Kahmann, Shenyu Nie, Guadalupe Vega,Shaoni Kar,Michał P. Nowak, Sebastian Maćkowski,Piotr Nyga,Caterina Ducati,Neil C. Greenham, Bettina V. Lotsch,Miguel Anaya,Samuel D. Stranks

Nature Communications(2024)

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摘要
Abstract Next-generation light-emitting applications such as displays and optical communications require judicious control over emitted light, including intensity and angular dispersion. To date, this remains a challenge as conventional methods require cumbersome optics. Here, we report highly directional and enhanced electroluminescence from a solution-processed quasi-2-dimensional halide perovskite light-emitting diode by building a device architecture to exploit hybrid plasmonic-photonic Tamm plasmon modes. By exploiting the processing and bandgap tunability of the halide perovskite device layers, we construct the device stack to optimise both optical and charge-injection properties, leading to narrow forward electroluminescence with an angular full-width half-maximum of 36.6° compared with the conventional isotropic control device of 143.9°, and narrow electroluminescence spectral full-width half-maximum of 12.1 nm. The device design is versatile and tunable to work with emission lines covering the visible spectrum with desired directionality, thus providing a promising route to modular, inexpensive, and directional operating light-emitting devices.
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