Electroadsorption Desalination Performance of Carbon Materials Derived from Coconut Shell without Membrane Separation

Lei Cao,Yun Li, Tiantian Zhou, Ling Gan,Haiou Song, Xiaoya Fang, Kaiqiang Shi, Yongwei Jiang, Xiajing Ge, Junwei Zhou

Desalination and Water Treatment(2024)

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Abstract
This study investigated coconut shells, an abundant and low-cost raw material, as the precursor for activated carbon preparation, and applied a carbonization activation method to prepare carbon materials under different activation conditions. The differences in the performance of biomass derived carbon materials as capacitive deionization (CDI) electrodes were studied under conditions of different activators, activator doses, and activation temperatures. Compared with commercial coconut shell activated carbon, studies have shown that biomass derived carbon electrodes obtained under the optimal preparation conditions of NaOH as the activator, a carbonizer to activator ratio of 1:3, and an activation temperature of 800 ℃ have an excellent electro adsorption performance and the potential to be used as a CDI electrode material. The salt adsorption capacity (SAC) of activated carbon made with coconut shell derived carbon materials after 20min of electro adsorption reached a maximum of 11.47mg/g. After 10 repeated uses, its SAC remained at the original 90.58%, demonstrating an excellent cycling stability.
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