Chinese Architecture Inspired Smart Roof Tile Integrating Radiation Cooling, Water Harvesting, and Energy Recycling

The development of new materials for resource and energy recycling has emerged as a primary focus in addressing global energy and environmental sustainability challenges. Inspired by traditional Chinese architecture, a smart roof tile (SRT) is scientifically designed, which incorporates hierarchical micro-nanostructured polyethylene/silica/barium sulfate composites (IH-PSB), semiconductor power generation modules, and LED chips. Leveraging the combined effects of surface and interface functionalities, the IH-PSB demonstrates exceptional sub-ambient cooling capabilities, resulting in its surface and bottom temperature being 5.4 °C and 12.1 °C lower than the ambient temperature, respectively. Additionally, the precisely controlled heterogeneous wettability, with a contact angle of approximately 151° and a roll-off angle of around 32°, allows the IH-PSB to efficiently condense moisture and transport droplets. Benefiting from the excellent radiation cooling performance and precisely controlled heterogeneous wettability, the IH-PSB exhibits remarkable passive sub-dewpoint cooling efficiency coupled with efficient water harvesting performance. During a one-month outdoor experiment, the IH-PSB operated stably and continuously without any electrical input, maintaining a mass flux ranging from ~23.2 to 50.0gm-2 h-1. Interestingly, the SRT system efficiently harnesses waste heat generated by the LEDs while simultaneously regulating their temperature effectively. The development and utilization of the SRT offer a sustainable, energy-efficient, and forward-thinking solution that addresses global water scarcity and energy crises.