Aza-[4 + 2] annulations of α-vinyl Morita-Baylis-Hillman adducts for regiodivergent synthesis of exomethylene-bearing azatricyclic compounds

Ye Liu, Chao-Xu Li, Chen Huang,Lei Zhu, Guo-Yin Xiong, Yu-Chao Zhu,Shilu Fan, Jian-Jun Dai,Hua Xiao

Organic Chemistry Frontiers（2024）

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摘要

Aza-[4 + 2] annulation reactions between α-vinyl Morita−Baylis−Hillman (MBH) adducts and cyclic imines have been developed, achieving regiodivergent synthesis of two distinct types of azatricyclic products. The process initiates with...

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