Magnetic anisotropy in single-crystalline antiferromagnetic Mn_2Au
arxiv(2024)
摘要
Multiple recent studies have identified the metallic antiferromagnet Mn_2Au
to be a candidate for spintronic applications due to apparent in-plane
anisotropy, preserved magnetic properties above room temperature, and
current-induced Néel vector switching. Crystal growth is complicated by the
fact that Mn_2Au melts incongruently. We present a bismuth flux method to
grow millimeter-scale bulk single crystals of Mn_2Au in order to examine the
intrinsic anisotropic electrical and magnetic properties. Flux quenching
experiments reveal that the Mn_2Au crystals precipitate below 550C,
about 100C below the decomposition temperature of Mn_2Au. Bulk Mn_2Au
crystals have a room-temperature resistivity of 16-19 μΩ-cm and a
residual resistivity ratio of 41. Mn_2Au crystals have a dimensionless
susceptibility on the order of 10^-4, comparable to calculated and
experimental reports on powder samples. Single-crystal neutron diffraction
confirms the in-plane magnetic structure. The tetragonal symmetry of Mn_2Au
constrains the ab-plane magnetic susceptibility to be constant, meaning that
χ_100=χ_110 in the low-field limit, below any spin-flop transition.
We find that three measured magnetic susceptibilities χ_100,
χ_110, and χ_001 are the same order of magnitude and agree with
the calculated prediction, meaning the low-field susceptibility of Mn_2Au is
quite isotropic, despite clear differences in ab-plane and ac-plane
magnetocrystalline anisotropy. Mn_2Au is calculated to have an extremely high
in-plane spin-flop field above 30 T, which is much larger than that of another
in-plane antiferromagnet Fe_2As (less than 1 T). The subtle anisotropy of
intrinsic susceptibilities may lead to dominating effects from shape,
crystalline texture, strain, and defects in devices that attempt spin readout
in Mn_2Au.
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