Remote enantioselective desymmetrization of cyclohexanone with carbonyl 1,2-transposition
Chem Catalysis(2024)
摘要
In this issue of Chem Catalysis, Ye and co-workers present a bisguanidinium-catalyzed method involving an intramolecular carbonyl 1,2-transposition for the remote enantioselective desymmetrization of prochiral cyclohexanone. The comprehensive mechanistic experiments, coupled with density functional theory (DFT) calculations, lay a robust foundation for future advancements in functional-group transposition.
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