Negatively enhanced thermopower near a Van Hove singularity in electron-doped Sr_2RuO_4
Physical Review Research(2024)
摘要
The layered perovskite Sr_2RuO_4 serves as a model material of the
two-dimensional (2D) Fermi liquid but also exhibits various emergent phenomena
including the non-Fermi-liquid (NFL) behavior under external perturbations such
as uniaxial pressure and chemical substitutions. Here we present the
thermoelectric transport of electron-doped system Sr_2-yLa_yRuO_4, in
which a filling-induced Lifshitz transition occurs at the Van Hove singularity
(VHS) point of y≈ 0.2. We find that the sign of the low-temperature
thermopower becomes negative only near the VHS point, where the NFL behavior
has been observed in the earlier work. This observation is incompatible with
either a numerical calculation within a constant relaxation-time approximation
or a toy-model calculation for the 2D Lifshitz transition adopting an elastic
carrier scattering. As a promising origin of the observed negatively enhanced
thermopower, we propose a skewed NFL state, in which an inelastic scattering
with a considerable odd-frequency term plays a crucial role to negatively
enhance the thermopower.
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