Flexoelectricity-enabled Modulation of Fermi Level in Graphene/PZT Heterostructure for Weak Pressure Signals Sensor

IEEE Sensors Journal(2024)

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Abstract
The flexoelectricity polarization of nanoscale dimensions has a natural advantage in realizing highly sensitive pressure sensors in two-dimensional. Further, as typical Two-dimensional material materials, graphene was often combined for pressure sensors. As the result of a high dielectric constant, PZT nanofilm could produce large surface polarization potential when subjected to external weak force. Then fermi level graphene on the surface of PZT film can be regulated by polarization electric field, which weak pressure signals sensor. We report on a novel graphene-based PZT pressure sensor with high sensitivity, fast response time, and weak pressure signals based on the flexoelectricity enhancement effect. Simulation of the Graphene/PZT composite structure by COMSOL Multiphysics and MATLAB indicates that the strain gradient of the PZT film is as high as 10 5 . Combining the high flexoelectricity coefficient of PZT with outstanding carrier transport of graphene, graphene-based PZT pressure sensor except high sensor expect exhibition highly sensitive, with an average sensitivity of 0.01 kPa -1 , a faster response time as 0.06s, and signal-to-noise(S/N) ratio is 61.9 dB in the range of pressure from 0.098 kPa to 9.8kPa. When compared with conventional pressure sensors, the sensors have orders of magnitude higher sensitivity. This Graphene/PZT-based pressure sensor will have great potentials for highly sensitive weak pressure signal detection.
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Key words
Graphene,PZT,Pressure sensor,Flexoelectricity,Fermi level,Carrier mobility
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