The polarisation fluctuation length scale shaping the superconducting dome of SrTiO_3

arxiv(2024)

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摘要
Superconducting domes, ubiquitous across a variety of quantum materials, are often understood as a window favorite for pairing opened by the fluctuations of competing orders. Yet, a quantitative understanding of how such a window closes is missing. Here, we show that inelastic neutron scattering, by quantifying a length scale associated with polar fluctuations, ℓ_0, addresses this issue. We find that the superconducting dome of strontium titanate definitely ends when ℓ_0 vanishes. Moreover, the product of ℓ_0 and the Fermi wavevector peaks close to the maximum critical temperature. Thus, this superconducting dome stems from the competition between the increase of the density of states and the unavoidable collapse of the quantum paraelectric phase, both induced by doping. The successful quantitative account of both the peak and the end of the superconducting dome implies a central role in the pairing mechanism played by the soft ferro-electric mode and its hybridisation with the acoustic branch. Such a scenario may also be at work in other quantum paraelectric materials, either bulk or interfaces.
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