Effect of operating conditions on the performance of riser reactor for oxidative coupling of methane

Particuology(2024)

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Abstract
Oxidative coupling of methane (OCM) is characterized by high temperature and strong heat released. A riser reactor is designed for the OCM process to improve gas-solid contacting and heat transfer. This work illustrates the effect of hydrodynamic conditions and feed gas composition on the performance of an OCM riser reactor. The findings suggest that oxidative reactions predominantly occur within the acceleration zone and developed flow zone. Furthermore, at the low superficial gas velocity accompanied by a high solid circulating rate, the C2 yield initially increases in the acceleration zone, followed by a decrease in the developed flow zone and deceleration zone. The optimal operating conditions are a specific region corresponding to the solids holdup ranges from 0.015 to 0.02. Moreover, the C2 yield can be elevated using an appropriate feed mixture.
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Key words
Oxidative coupling of methane,Riser,Hydrodynamics,Solids holdup
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