Sequential proton coupled electron transfers from a tetraruthenium polyoxometalate in photochemical water oxidation

Elena Rossin,Marcella Bonchio,Mirco Natali,Andrea Sartorel

Sustainable Energy & Fuels（2024）

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摘要

The tetraruthenium polyoxometalate {RuIV(H2O)4(μ-OH)2(μ-O)4[SiW10O36]2} (Ru4POM) shows multiple oxidative proton coupled electron transfer (PCET) events in a [Ru(bpy)3]2+ / S2O82- photochemical cycle for catalytic water oxidation, with electrons conveyed to the...

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