Friction, Mineralogy, and Microstructures: How Complex is the Brittle Deformation of Faults?

Faults accommodate most of the brittle deformation that occurs in the lithosphere  through a spectrum of fault slip behaviours including, but not limited to, seismic and aseismic slip. The rocks deforming inside the core of the faults are the main actors that control the modality of slip and thus their mechanical properties are a key subject of study that is carried out through experimental investigation. The most relevant characterization is that of friction, a property that commensurates the resistance to shear motion of the rocks. Nevertheless, friction is not an intrinsic constant feature of the investigated materials. It is instead modulated by several attributes and external factors. For instance, the rate and state constitutive framework describes the sensitivity of friction to the sliding velocity, proving a successful theory to quantify the potential of the onset of dynamic instabilities and seismic slip in natural faults. Several works have also demonstrated that the frictional properties of the same material can dramatically change as function of the fabric (textural, geometrical attributes of the deforming rock). It is therefore evident that brittle deformation of rocks cannot be assessed in isolation of the conditions at which the phenomenon is measured. To fully understand the complex bulk behaviour of a deforming fault zone material we must investigate the interaction of several scale-dependent mechanisms that are active from the grain-scale up to the entire fault zone thickness. In this work we present the results of several case-studies that cover relevant lithotypes: anhydrite-dolomite, quartz-calcite-mica, lizardite-magnetite mixtures. These studies collect more than 60 friction experiments performed on BRAVA biaxial apparatus (INGV, Italy), presented here by associating the analysis of mechanical data with the analysis of rock microstructures. This joined investigation highlights the mechanisms that control rock friction: cataclasis, crystal plasticity, pressure-solution, grain-boundary sliding, cementation, and indentation. We also show the emergence of complex slip behaviours (experimental fault stability) as function of the coexistence of processes with different timescales and explained by the spatial arrangement of the mineral phases in the fault core. Our results shed light on the origin of the macroscopic frictional properties of fault rocks, stressing the fact that they are not a characterising property but rather the observable of a complex, dynamic, and highly non-linear system.