Coconut-Solid-Waste-Derived Hard-Carbon Anode Materials for Fast Potassium Ion Storage

Yi Ma,Wenhao Liu, Wenhan Liu, Guangwan Zhang,Yu Wang,Haokai Wang,Wei Chen,Meng Huang,Xuanpeng Wang

COATINGS(2024)

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摘要
Hard carbon, which features recyclability, low costs, and environmental friendliness, is an attractive anode material for K+ storage. Nevertheless, the state-of-the-art hard carbon is still unsatisfactory due to its poor multiplication performance and unclear energy storage mechanism. In this study, a one-pot carbonisation method using coconut solid waste biomass is applied to obtain high-performance hard-carbon (CHC) anode materials. The microstructure and electrochemical properties of the CHC are investigated at different carbonisation temperatures (1100-1500 degrees C). The CHC materials prepared at 1300 degrees C (CHC1300) have a high capacity of 265.8 mAh g-1 at a current density of 25 mA g-1 and a superior cyclability of 1000 cycles at 1.0 A g-1 with a capacity retention of 96.6%. This approach, referred to as the "biomass-to-application" strategy, holds promise for advancing the development of cost-effective and sustainable KIBs.
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关键词
potassium-ion batteries,anode materials,hard carbon,coconut,biomass
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