High-performance antibacterial tight ultrafiltration membrane constructed by co-deposition of dopamine and tobramycin for sustainable high-salinity textile wastewater management
DESALINATION(2024)
摘要
High-salinity textile wastewater is a pressing environmental concern, urgently requiring the appropriate treatment. Sustainable management of high-salinity textile wastewater via fractionation of the existing dyes and inorganic salts (NaCl) using selective separation membranes is a key approach to address this detrimental concern. Herein, tight composite ultrafiltration membranes with impressive antibacterial function were constructed using one-step co-deposition of dopamine and tobramycin on the porous substrate to fractionate the dyes and NaCl. Triggered by ammonia persulfate, the polydopamine/tobramycin coating layer imparts the fabricated composite ultrafiltration membranes with tight surface structure and narrow pore size distribution, enabling effective dyes/salts fractionation. Specifically, the tight composite ultrafiltration membrane with a molecular weight cutoff of 3692 Da experienced a > 98.0 % rejection against various reactive dyes (molecular weight: <1000 Da) with nearly complete salt transmission (<0.8 % NaCl rejection), demonstrating an effective fractionation of dyes and salts. Additionally, the incorporated tobramycin as a broad-spectrum antibiotic endowed the tight composite ultrafiltration membrane with a sufficient inhibition efficiency (i.e., 100 %) against E. coli bacteria in a short-time contact (i.e., 3 min). Thereby, the tight composite ultrafiltration membrane constructed by fast co-deposition of dopamine and tobramycin established an unparalleled platform technology for sustainable resource recovery (dyes or salts) from high-salinity textile wastewater.
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关键词
Tight ultrafiltration membranes,Polydopamine coating,Tobramycin,Antibacteria,High-salinity textile wastewater
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