Visible‐light Induced Cerium‐catalyzed N‐Demethylation of N‐Methyl Amides under Air Conditions

Qing‐Hu Teng, Greg Sun,Huang Fang-Ping, Kai Wang,Fu‐Pei Liang

Advanced Synthesis & Catalysis（2023）

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摘要

Abstract A visible‐light induced cerium‐catalyzed N ‐demethylation of N ‐methyl amides under air atmosphere to the corresponding of N ‐demethylated amides is presented. Upon irradiation the excited states of [Ce IV Cl n ] 2− are able to activate N ‐methyl amides. This reaction provides a methodology to cleave the C−N bond of amides under air conditions. magnified image

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关键词

cerium‐catalyzed,‐demethylation

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