NO formation by N2/O2 plasma catalysis: The impact of surface reactions, gas-phase reactions, and mass transport

Brian N. Bayer,Peter J. Bruggeman,Aditya Bhan

Chemical Engineering Journal（2024）

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摘要

•Silver catalyzes NO formation from plasma-derived N radicals with high selectivity.•Rates of N conversion to NO on the surface are determined by rates of mass transfer processes.•Consumption of N in the gas phase limits the ability of N to diffuse to the surface and react to form NO.

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关键词

Plasma catalysis,Molecular beam mass spectrometry,Nitrogen fixation,Radical chemistry,Reaction–diffusion

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