Investigation of catalytic activation of peroxydisulfate on cu-doped mesoporous silica-based particles (Cu-BMS) for efficient degradation of methylene blue

CATALYSIS COMMUNICATIONS(2024)

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摘要
The Cu-doped mesoporous silica-based particles (Cu-BMS) were prepared using an evaporation-induced selfassembly sol-gel procedure as a heterogeneous catalyst for the activation of peroxydisulfate (PDS). The formation of well-organized mesoporous structures with amorphous nature and high surface area of 286 m(2)/g was demonstrated. The catalytic activity of Cu-BMS in the degradation of Methylene Blue (MB) and the effects of operating parameters, including Cu-BMS dosage, initial PDS amount, initial MB concentration, temperature and initial pH, were investigated in details. The Cu-BMS demonstrated a remarkable catalytic activity (93.5% degradation efficiency within 60 min) and good stability.
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关键词
Mesoporous catalyst,Persulfate activation,Advanced oxidation process (AOP),Organic pollutant
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