Engineering a defect-rich Prussian blue analog composite for enhanced Cs+ removal performance
CHEMICAL COMMUNICATIONS(2024)
Abstract
Using a novel, irregular honeycombed N-doped porous carbon (NPC) as a support and defect inducer, defect-rich Zn-PBA was formed in situ and evenly anchored on the surface of NPC to obtain a defect-rich Zn-PBA/NPC composite. This composite demonstrated an ultrafast Cs+ adsorption rate that reached equilibrium within 60 s as well as excellent adsorption capacity, stability and reusability. The adsorption mechanism indicated that Cs+ was quickly adsorbed via the defect sites close to the Zn-PBA crystal face accompanied by K(OH2)(+) elimination.
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