Observation of Parallel Intersystem Crossing and Charge Transfer-state Dynamics in [Fe(bpy)₃]²⁺ from Ultrafast 2D Electronic Spectroscopy

Angela Lee,Minjung Son,Mawuli Deegbey,Matthew D Woodhouse, S. R. Hart, Hayden F Beissel,Paul T Cesana,Elena Jakubı́ková,James K. McCusker,Gabriela S. Schlau‐Cohen

Chemical Science（2023）

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摘要

Ultrafast two-dimensional electronic spectroscopy, in conjunction with DFT calculations, revealed parallel pathways for the earliest stages of charge transfer-state evolution in the prototypical first-row transition metal complex [Fe(bpy) 3 ] 2+ .

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关键词

parallel intersystem crossing,transfer-state,transfer-state

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Observation of Parallel Intersystem Crossing and Charge Transfer-state Dynamics in [Fe(bpy)3]2+ from Ultrafast 2D Electronic Spectroscopy

Observation of Parallel Intersystem Crossing and Charge Transfer-state Dynamics in [Fe(bpy)₃]²⁺ from Ultrafast 2D Electronic Spectroscopy