Topotactic transformation of metal–organic frameworks to iron-based catalysts for the direct hydrogenation of CO₂ to olefins

Qing Yang,Ruifeng Wang,Xiong Zhang, Shi fu Wang,Qi Yu,Xiong Su,Xuning Li,Yanqiang Huang

Catalysis Science & Technology（2023）

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摘要

The effects of different metal promoters in MFe/C catalysts on CO 2 hydrogenation were investigated and specific Fe sites within Fe 5 C 2 (sites II and III) were found positively correlated to the O/P ratio and olefin selectivity.

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direct hydrogenation,catalysts,metal–organic frameworks,topotactic transformation,iron-based

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Topotactic transformation of metal–organic frameworks to iron-based catalysts for the direct hydrogenation of CO2 to olefins

Topotactic transformation of metal–organic frameworks to iron-based catalysts for the direct hydrogenation of CO₂ to olefins