Dearomative intermolecular [2 + 2] photocycloaddition for construction of C(sp³)-rich heterospirocycles on-DNA

Gary A. Molander,Longbo Li,Bianca Matsuo,Guillaume Levitre,Edward J. McClain,Eric A. Voight,Erika A Crane

Chemical Science（2023）

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摘要

Diverse DNA-encoded libraries of complex and novel sp 3 -rich spirocycles were achieved using a versatile and operationally simple visible light-mediated intermolecular [2 + 2] cycloaddition.

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关键词

heterospirocycles,photocycloaddition,on-dna

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Dearomative intermolecular [2 + 2] photocycloaddition for construction of C(sp3)-rich heterospirocycles on-DNA

Dearomative intermolecular [2 + 2] photocycloaddition for construction of C(sp³)-rich heterospirocycles on-DNA