Site-selective C−H difunctionalization of N-alkyl activated azaarenes via the synergistic catalysis of graphene oxide and visible light

Dehao Duan,Haiping He, Wenping Ding,Dongcheng Yi, Yongzhen Lai, Aiwen Huang,Jie Liu, Wen−Fa Wu,Xiangjun Peng

Organic chemistry frontiers（2023）

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Abstract

Employing heterogeneous cocatalyst-graphene oxide, light-induced site-selective difunctionalizations of pyridiniums/quinoliniums provided straightforward synthetic route toward C4- and C2-phosphonated pyridinone/quinolinone/quinolone cores under air atmosphere.

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Key words

graphene oxide,azaarenes,synergistic catalysis,site-selective,n-alkyl

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