Towards frustration in Eu(ii) Archimedean tessellations

Hua Chen, Anna S. Manvell, Maiusz Kubus,Maja A. Dunstan, Giulia Lorusso,David Gracia, Mike S. B. Jørgensen, Søren Kegnæs, F. Wilhelm, А. Рогалев,Marco Evangelisti, Kasper S. Pedersen

Chemical Communications（2023）

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摘要

Self-assembly of trans-{EuI2} nodes and ditopic ligands leads to isoreticular 2D frameworks featuring a rare, non-kagome Archimedean tessellation. The topology and intra-layer Eu(II)-Eu(II) antiferromagnetic interactions provide the prerequisites for geometrical spin frustration, which, due to the spin state degeneracy, is key for novel phenomena such as enhanced magnetic refrigeration.

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关键词

archimedean tessellations,eu<scp>ii</scp>,frustration

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