SmI₂-mediated intermolecular addition–elimination of piperidine and pyrrolidine N-α-radicals with arylacetylene sulfones

Changhong Liu, Jiangming Guo,Xin Li,Jian-Ting Sun,Bang‐Guo Wei,Chang‐Mei Si

Chemical Communications（2022）

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摘要

An efficient approach to access α-arylacetylene-substituted pyrrolidine and piperidine derivatives has been developed through a samarium diiodide-mediated addition-elimination process of pyrrolidine and piperidine N-α-radicals with arylacetylene sulfones.

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intermolecular addition–elimination,piperidine,pyrrolidine,sulfones

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SmI2-mediated intermolecular addition–elimination of piperidine and pyrrolidine N-α-radicals with arylacetylene sulfones

SmI₂-mediated intermolecular addition–elimination of piperidine and pyrrolidine N-α-radicals with arylacetylene sulfones