Peak-like three-dimensional CoFe 2 O 4 /carbon nanotube decorated bamboo fabrics for simultaneous solar-thermal evaporation of water and photocatalytic degradation of bisphenol A
Journal of Materials Science & Technology(2024)
Abstract
Catalytic CoFe 2 O 4 and solar-thermal carbon nanotube decorated bamboo fabrics (CCBF) are fabricated for integrating efficient solar steam generation from wastewater with catalytic degradation of its organic contaminants. Thanks to the numerous porous channels and polar groups of bamboo fabric and the efficient solar-thermal energy conversion of black carbon nanotubes, the porous and hydrophilic CCBF exhibits fast upward transport of water, efficient solar light absorption, and high solar-thermal energy conversion efficiency. The decorated CoFe 2 O 4 not only enhances the solar-thermal energy conversion efficiency of CCBF but also activates potassium peroxymonosulfate to generate abundant highly active species for catalytic degradation of bisphenol A (BPA). Furthermore, folding the CCBF into a peak-like 3D evaporator can enhance solar energy utilization, and gain environmental energy for promoting solar-thermal water evaporation and catalytic degradation performances. The 3D CCBF evaporator achieves a water evaporation rate of 2.72 kg m -2 h -1 under 1-sun irradiation. Meanwhile, 100% of the BPA in the seawater can be degraded within 10 min. An exceptional high purification efficiency of 27.72 kg m -2 h -1 is achieved with the 3D evaporator during a long-term treatment of BPA-containing seawater under 1-sun irradiation. This work demonstrates efficient purification of seawater/wastewater with both metal ions and organic pollutants by simultaneous solar-thermal evaporation of water and catalytic degradation of organic pollutants. (c) 2023 Published by Elsevier Ltd on behalf of The editorial office of Journal of Materials Science & Technology.
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Key words
Solar-thermal water evaporation,Seawater desalination,Catalytic degradation,Carbon nanotubes
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