Generation of Ultrafast Laser Pulses at the SXP Instrument of the European XFEL

Patrik Grychtol, Ekaterina Tikhodeeva, Marcus Seidel, Christoph M. Heyl, Vahagn Vardanyan, David Doblas-Jiménez,Serguei Molodtsov,Manuel Izquierdo

2023 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)(2023)

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摘要
At the European X-ray Free Electron Laser (XFEL) facility a new instrument, the Soft X-ray Port (SXP), is currently under commissioning [1]. It is primarily designed for time- and spin-resolved X-ray photo-electron spectroscopy (TR-XPES), but investigations of complex chemical and bio-inorganic molecular systems with fluorescence spectroscopy as well as research on highly charged ions are also envisioned [2]. SXP is located downstream of the SASE 3 soft X-ray undulator system providing ultrafast photon pulses with variable polarization in the energy range between 260 eV and 3000 eV, at MHz repetition rates. Up to $10^{12}$ photons per pulse will be focus at the interaction region in a micrometer spot size resulting in an intensity of more than $10^{18}\mathrm{W}/\text{cm}^{2}$ . These outstanding specifications will enable the complete electronic, chemical and atomic characterization of solids, surfaces and interfaces using TR-XPES. For this purpose, two powerful pump-probe lasers operating in a broad spectral range from the mid-infrared to the ultraviolet region will be available. Herriott-type multi pass cells (MPC) will be used to compress their pulses into the few femtosecond range paving the way for ultrafast time-resolved investigations at the SXP instrument combining intense and tunable soft X-rays with versatile optical laser capabilities. Fig. 1 On the left, typical laser spectra before and after passing the herriott multi pass cell. On the right, autocorrelation measurements of the original and compressed laser pulses showing a reduction in pulse lengths from 300 fs to about 30 fs.
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broad spectral range,complex chemical,compressed laser pulses,energy range,European X-ray Free Electron Laser,European XFEL,femtosecond range,fluorescence spectroscopy,herriott-type multipass cells,highly charged ions,intense X-rays,interaction region,left laser spectra,MHz repetition rates,micrometer spot size,original laser pulses,powerful pump-probe lasers,pulse lengths,SASE 3 soft X-ray undulator system,Soft X-ray Port,SXP instrument,time 30.0 fs to 300.0 fs,TR-XPES,tunable soft X-rays,typical laser spectra,ultrafast Laser pulses,ultrafast photon pulses,ultrafast time-resolved investigations,ultraviolet region,variable polarization,versatile optical laser capabilities,X-ray photo-electron spectroscopy
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