Theoretical Study of Multicascade Raman Microlasers Based on TeO₂-WO₃-Bi₂O₃ Glass

The development and investigation of miniature narrow-line coherent light sources based on microresonators with low-power-consumption whispering gallery modes (WGMs) is an actual trend in modern photonics. Raman WGM microlasers can operate at wavelengths inaccessible to traditional laser media and provide a huge pump frequency tuning range. Here, we propose and theoretically study multicascade Raman microlasers based on soft tellurite TeO2-WO3-Bi2O3 glass WGM microresonators (microspheres) which can operate in the near-IR and mid-IR with the pump in the telecommunication range. Thanks to a large Raman gain (120 times exceeding the maximum Raman gain of silica glass) and a huge Raman frequency shift of 27.5 THz for this glass, the Raman waves at 1.83 mu m, 2.21 mu m, 2.77 mu m, and 3.7 mu m in the first, second, third, and fourth cascades, respectively, are theoretically demonstrated with a pump at 1.57 mu m. We analyze in detail the influence of different factors on the characteristics of the generated Raman waves, such as microsphere diameters, Q-factors, pump powers, and detuning of the pump frequency from exact resonance. We also solve a thermo-optical problem to show that the temperature of a soft glass microresonator heated due to partial thermalization of pump power remains below the glass transition temperature. To the best of our knowledge, mid-IR tellurite glass Raman WGM microlasers have not been studied before.