Zeolite-mediated hybrid Cu+/Cu0 interface for electrochemical nitrate reduction to ammonia

Jiabao Lv,Angjian Wu,Liang Wang,Yunhao Zhong,Zhihao Zeng,Qunxing Huang,Xiaoqing Lin,Hao Zhang,Shaojun Liu,Qian Liu,Songqiang Zhu,Xiaodong Li,Jianhua Yan,Zhifu Qi,Hao Bin Wu

Journal of Energy Chemistry（2023）

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摘要

The Cu+/Cu0 active site was well maintained by zeolite mediated under negative potential, thus achieving the ammonia synthesis activity of 41.65 mg h−1 cm−2 with ∼100% Faradaic efficiency.

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关键词

Electrochemical nitrate reduction reaction, Ammonia synthesis, In-situ Raman spectroscopy, Zeolite, Density functional theory

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