Chirality Transfer Intramolecular Pauson–Khand Reaction with N–C Axially Chiral Sulfonamides Bearing an Ene–Yne Structure

Ryohei Kasahara,Tatsuya Toyoda,Sota Fukasawa, Aoi Takeuchi,Azusa Sato,Akiko Hori,Osamu Kitagawa

Organic letters（2023）

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摘要

An intramolecular Pauson-Khand reaction with enantioenriched N-C axially chiral -allyl--(2-alkynylphenyl)sulfonamide derivatives proceeded with complete chirality transfer from axial chirality ( configuration) to central chirality ( configuration), affording chiral nitrogen-containing tricyclic compounds (tetrahydrocyclopentaquinolin-2-one derivatives).

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