Coulomb potential screening via charged carriers and charge-neutral dipoles/excitons in two-dimensional case

arXiv (Cornell University)(2023)

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摘要
With the shrink of dimensionality, Coulomb interaction displays a distinct role owing to the reduced dielectric screening in out-of-plane direction. Apart from the dielectric screening, the free charge carriers and/or dipoles can also make nonnegligible contribution to Coulomb interaction. While the Thomas Fermi model is effective in describing charge carrier screening in three dimensions, the extent of screening to two-dimension resulting from charge-neutral dipoles and carriers remains quantitatively unclear. To address this gap, we present a simple analytical solution based on linear response theory, offering a comprehensive depiction of the Coulomb screened potential in both 2D and 3D systems, where screening effects from both charge carriers and charge-neutral dipoles are addressed. Our work provides a handy tool for directly analysing and evaluating Coulomb interaction strength in atomically thin materials and particularly in the context of electronic and optoelectronic engineering. As a demonstration, we utilize the derived modified Coulomb potential for the exciton system to estimate the exciton binding energy variation arising from exciton density fluctuation and the temperature dependent exciton polarizability, yielding excellent agreement with the experimental and computational findings.
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关键词
coulomb potential screening,dipoles/excitons,dipoles/excitons,charge-neutral,two-dimensional
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