Magnetic Imaging and Domain Nucleation in CrSBr Down to the 2D Limit

Recent advancements in 2D materials have revealed the potential of van der Waals magnets, and specifically of their magnetic anisotropy that allows applications down to the 2D limit. Among these materials, CrSBr has emerged as a promising candidate, because its intriguing magnetic and electronic properties have appeal for both fundamental and applied research in spintronics or magnonics. In this work, nano-SQUID-on-tip (SOT) microscopy is used to obtain direct magnetic imaging of CrSBr flakes with thicknesses ranging from monolayer (N = 1) to few-layer (N = 5). The ferromagnetic order is preserved down to the monolayer, while the antiferromagnetic coupling of the layers starts from the bilayer case. For odd layers, at zero applied magnetic field, the stray field resulting from the uncompensated layer is directly imaged. The progressive spin reorientation along the out-of-plane direction (hard axis) is also measured with a finite applied magnetic field, allowing evaluation of the anisotropy constant, which remains stable down to the monolayer and is close to the bulk value. Finally, by selecting the applied magnetic field protocol, the formation of Neel magnetic domain walls is observed down to the single-layer limit. Using direct magnetic imaging of CrSBr, a van der Waals material 2D antiferromagnet, it is demonstrated that the magnetic anisotropy and moment density are nearly preserved down to the monolayer. These images reveal the formation of Neel magnetic domain walls down to the monolayer. This material shows remarkable stability even for monolayer exposed to air.image