Effects of F- on the electrochemical properties and electrodeposition nucleation mechanism of Ce(III) in LiCl-KCl melts

Xiaorui Xu, Tianxing Shi, Yuncong Ding,Xinyu Zhang,Jia Song,Hong Zhang,Yafei Wang,Wentao Zhou,Shaoqiang Guo

Journal of Electroanalytical Chemistry（2023）

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摘要

•The effect of F− on the electrochemical properties of Ce(III) was investigated.•F− was found to react with [CeCl6]3− to [CeCl5F]3−.•The addition of F− increased the electrochemical polarization of Ce(III)/Ce reaction.•The nucleation mode of Ce(III) was changed with the addition of F−.

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关键词

Electrochemical properties, Coordination competition, F-ions, Electrodeposited nucleation of Ce(III), Uranium dendrites

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