Tunable catalysis by reversible switching between Ru(III) single sites and Ru0 clusters in solid micelles

Qiyan Wang, Catarina M. De Brito Mendes,Olga V. Safonova,Walid Baaziz,César A. Urbina-Blanco,Dan Wu,Maya Marinova,Ovidiu Ersen,Mickael Capron,Andrei Y. Khodakov,Mark Saeys,Vitaly V. Ordomsky

JOURNAL OF CATALYSIS（2023）

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摘要

•Ru(III) sites in solid micellar catalyst can be reversible switched to Ru0 clusters.•Ru(III) single-sites selectively catalyze the hydrogenation of functional groups.•Ru0 nanoclusters in contrast are very active for hydrogenating aromatic rings.

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关键词

Ruthenium,Solid Micelles,Single-site,Cluster,Switching Catalysis,Arene hydrogenation

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