Elimination of Chirality in Three-Dimensionally Confined Open-Access Microcavities.

Nanomaterials (Basel, Switzerland)(2023)

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摘要
The emergent optical activity (OA) caused by anisotropic light emitter in microcavities is an important physical mechanism discovered recently, which leads to Rashba-Dresselhaus photonic spin-orbit (SO) coupling. In this study, we report a sharp contrast of the roles of the emergent OA in free and confined cavity photons, by observing the optical chirality in a planar-planar microcavity and its elimination in a concave-planar microcavity, evidenced by polarization-resolved white-light spectroscopy, which agrees well with the theoretical predictions based on the degenerate perturbation theory. Moreover, we theoretically predict that a slight phase gradient in real space can partially restore the effect of the emergent OA in confined cavity photons. The results are significant additions to the field of cavity spinoptronics and provide a novel method for manipulating photonic SO coupling in confined optical systems.
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关键词
organic microcrystal,spin-orbit coupling,microcavity
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