Structural and reactive evolution of oxidatively grafted Pd catalysts on MnO 2 for the low-temperature oxidation of CO.

Jacklyn N Hall,A Jeremy Kropf,Uddhav Kanbur,Fulya Dogan,Carly Byron,Jianguo Wen,Massimiliano Delferro,David M Kaphan

Chemical communications (Cambridge, England)（2023）

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摘要

Isolated Pd atoms supported on high surface area MnO, prepared by the oxidative grafting of (bis(tricyclohexylphosphine-palladium(0)), catalyze (>50 turnovers, 17 h) the low temperature (≤325 K) oxidation of CO (7.7 kPa O, 2.6 kPa CO) with results of / and spectroscopic characterization signifying a synergistic role of Pd and MnO in facilitating redox turnovers.

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