Refining reaction kinetics of butadiene hydrogenation on zeolite-confined palladium clusters

Yi Wang,Qiao Yuan,Lihua Shi,Zhibing Chen,Xiaoling Mou, Menglu Li, Jingwei Dai,Xiangen Song,Ronghe Lin,Yunjie Ding

Molecular Catalysis（2023）

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摘要

•Pd clusters confined in ZSM-5 and supported on the outer surfaces were prepared.•Pd@ZSM-5 exhibited much improved butenes selectivity but lower hydrogenation activity.•The detailed reaction dynamics of hydrogenation and isomerization were studied.•The kinetic origin of high selectivity patterns on Pd@ZSM-5 was revealed.

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关键词

13-Butadiene Confinement effect, Hydrogenation Palladium Reaction kinetics

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