PolySchiff based self-healing solid-state electrolytes for lithium ion battery

Yuli Wang,Zonglei Wang, Bihui Jin,Dezhan Ye,Wuhou Fan,Xianke Ye

European Polymer Journal（2023）

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Abstract

•Dynamic imine bonds endow SPEs with self-healing function at room temperature.•The vitrimers SPEs with lower cross-linking degree show a lower Tg.•The σ increase with the dropping cross-linking degree and succinonitrile (SN) addition.•The electrochemical window was widened with SN addition, up to 5.1 V vs. Li/Li+.

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Key words

Polymer electrolytes, Self-healing, Reversible covalent bonds, Dynamic imine bonds

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