Response of axial nitrogen coordination engineering to cobalt based molecular environmental catalysts for selective reduction of CO2

Honghong Lyu,Jian Zhao,Boxiong Shen,Zhiqiang Wang,Shuna Jia

Chemical Engineering Journal（2023）

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摘要

•Three N-doped CNTs provide different coordination environments for CoPc.•Different types of axial coordination N adjust the electronic state of CoPc.•Donor amino axial coordination N increase TOF of CoPc for CO2RR.•Withdrawing pyridine axial coordination N increase FECO of CoPc for CO2RR.•Different types of axial coordination N adjust the CO2RR Gibbs free energy.

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关键词

CO2RR, CoPc, Axial coordination N, Pyridine Cyanobenzene Aminobenzene

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