Effect of boron and nitrogen modulation in metal atoms anchoring on flower-like carbon superstructure for efficient ammonia electrosynthesis

Yanchao Zhao,Shuo Zhang,Cong Han,Qian Lu,Qiuju Fu,Huimin Jiang,Lingzhi Yang,Yanlong Xing,Qiuju Zheng,Jianxing Shen,Liting Yan,Xuebo Zhao

Chemical Engineering Journal（2023）

引用 3|浏览6

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摘要

•MBON-1 with flower-like superstructure was synthesized by one-step method.•Fe-B/N-C was achieved by a high-temperature calcination process of Fe-MBON-1.•Fe with atomic-level dispersion on the flower-like superstructure was obtained.•Fe-B/N-C materials exhibit excellent catalytic activity and stability for NRR.•The effect of boron and nitrogen modulation was studied by DFT calculations.

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关键词

Single atom catalyst,Three-dimensional nanoflowers,Electrocatalytic nitrogen reduction reactions,Boron and nitrogen co-doped carbon

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