Full-exposed Cu site of Cu2O-(1 0 0) driven high ethylene selectivity of carbon dioxide reduction

Yilong Dong,Xingcheng Ma,Zhaoyong Jin, Xiaochun Xu,Tianyi Xu,Dantong Zhang,Xiaoqiang Cui

Applied Surface Science（2024）

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Abstract

The facet-dependent electrocatalytic reduction of CO2 to C2H4 on various Cu2O nanostructures was systematically investigated. The (100) facet with full-exposed Cu sites is favorable for *CO–*CO coupling with enhanced adsorption of *CO intermediates, resulting in the conducive conversion of CO2 into C2H4.

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Key words

Electrochemical CO2 reduction reaction,Cuprous oxide,DFT calculation,C2H4 production,Facet effect

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