Laser-based angle-resolved photoemission spectroscopy with micrometer spatial resolution and detection of three-dimensional spin vector

Takuma Iwata, T. Kousa, Y. Nishioka, K. Ohwada, K. Sumida, E. Annese, M. Kakoki,Kenta Kuroda,H. Iwasawa, M. Arita,S. Kumar, A. Kimura, K. Miyamoto, T. Okuda

SCIENTIFIC REPORTS(2024)

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Abstract
We have developed a state-of-the-art apparatus for laser-based spin- and angle-resolved photoemission spectroscopy with micrometer spatial resolution (mu-SARPES). This equipment is realized by the combination of a high-resolution photoelectron spectrometer, a 6 eV laser with high photon flux that is focused down to a few micrometers, a high-precision sample stage control system, and a double very-low-energy-electron-diffraction spin detector. The setup achieves an energy resolution of 1.5 (5.5) meV without (with) the spin detection mode, compatible with a spatial resolution better than 10 mu m. This enables us to probe both spatially-resolved electronic structures and vector information of spin polarization in three dimensions. The performance of mu-SARPES apparatus is demonstrated by presenting ARPES and SARPES results from topological insulators and Au photolithography patterns on a Si (001) substrate.
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Key words
photoemission spectroscopy,spin,laser-based,angle-resolved,three-dimensional
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