A Composite Gas-Phase Explosives Sensor with Frequency-Resistance Dual-Signal Display Based on Surface Acoustic Wave
ACS APPLIED ELECTRONIC MATERIALS(2023)
摘要
The surface acoustic wave (SAW) technology has been widely used for hazardous gas detection, but the low sensitivity, poor selectivity, long response/recovery time, and signal "false positives" of the sensors have limited its application for gas -phase explosives detection. In this paper, a composite gas-phase explosives sensor with frequency-resistance dual-signal display was designed by transferring 25 layers of graphene (rGO) in the sensing area of the SAW device and coupling p-aminothiophenol (PATP)-modified gold nanoparticles (AuNPs). The rGO:AuNP/ PATP-SAW sensor shows signal response from two signal dimensions, frequency and resistance, to 0.1-80 ppm TNT gas with a low detection limit (DL) of 41.2 ppb. The composite sensor has a short response/recovery time (9.8 s/27.1 s) with good selectivity, repeatability, and stability. The excellent gas-sensitive performance of the rGO:AuNP/PATP-SAW sensor was attributed to the fact that PATP provides a large number of selective capture groups, which are enriched in the sensing area by the presence of multiple strong interactions with 2,4,6-trinitrotoluene (TNT) molecules. This work will provide scientific guidance for the engineering promotion of surface acoustic wave gas-phase explosives sensors.
更多查看译文
关键词
rGO,SAW device,TNT sensing,frequency-resistance,PATP
AI 理解论文
溯源树
样例
生成溯源树,研究论文发展脉络
Chat Paper
正在生成论文摘要