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Mechanism of ion track formation in silicon by much lower energy deposition than the formation threshold

H. Amekura,K. Narumi,A. Chiba, Y. Hirano, K. Yamada,S. Yamamoto, N. Ishikawa,N. Okubo, M. Toulemonde, Y. Saitoh

PHYSICA SCRIPTA(2023)

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Abstract
Mechanism of the ion track formation in crystalline silicon (c-Si) is discussed, particularly under 1-9 MeV C-60 ion irradiation. In this energy region, the track formation was not expected because the energy E was much lower than the threshold of E (th) = 17 MeV determined by extrapolation from higher energy data in the past literature. The track formation is different between irradiations of C-60 ions and of monoatomic ions: The tracks were observed under 3 MeV C-60 ion irradiation but not under 200 MeV Xe ions, while both the irradiations have the same electronic stopping (S (e)) of 14 keV nm(-1) but much higher nuclear stopping (S (n)) for the former ions. The involvement of S (n) is suggested for the C-60 ions. While the inelastic thermal spike (i-TS) calculations predict that the high energy monoatomic ion irradiation forms the tracks, the tracks have never been experimentally detected, suggesting quick annihilation of the tracks by highly enhanced recrystallization in c-Si. Exceptions are C-60 ions of 1-9 MeV, where the track radii are well reproduced by the i-TS theory with assuming the melting transition. Collisional damage induced by the high S (n) from C-60 ions obstructs the recrystallization in c-Si. Then the tracks formed by the melting transition survive against the recrystallization. This is a new type of the synergy effect between S (e) and S (n), different from the already-known mechanisms, i.e., the pre-damage effect and the unified thermal spike. While c-Si was believed as a radiation-hard material in the S (e) regime with high S (e) threshold, this study suggests that c-Si has a low S (e) threshold but with efficient recrystallization.
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Key words
C-60 ion,ion track,swift heavy ion,silicon,synergy effect,track recrystallization
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