Unusual magnetotransport and anomalous Hall effect in quasi-two-dimensional van der Waals ferromagnet Fe_4GeTe_2
arxiv(2023)
摘要
Fe_4GeTe_2, an itinerant vdW ferromagnet (FM) having Curie temperature
(T_C) close to room temperature (∼ 270 K), exhibits another transition
(T_SR ∼ 120 K) where the easy axis of magnetization changes from
in-plane to the out-of-plane direction in addition to T_C. Here, we have
studied the magnetotransport in a multilayer Hall bar device fabricated on 300
nm Si/SiO_2 substrate. Interestingly, the zero field resistivity shows a
negligible change in resistivity near T_C unlike the typical metallic FM,
whereas, it exhibits a dramatic fall below T_SR. Also, the resistivity
shows a weak anomaly at T ∼ 38 K (T_Q), below which the resistivity
shows a quadratic temperature dependence according to the Fermi liquid
behavior. Temperature-dependent Hall data exhibits important consequences. The
ordinary Hall coefficient changes sign near T_SR indicating the change in
majority carriers. In a similar manner, the magnetoresistance (MR) data shows
significantly large negative MR near T_SR and becomes positive below T_Q.
The observations of anomaly in the resistivity, sign-change of the ordinary
Hall coefficient and maximum negative MR near T_SR, together suggest a
possible Fermi surface reconstruction associated with the spin reorientation
transition. Furthermore, analysis of the Hall data reveals a significant
anomalous Hall conductivity (AHC) from ∼ 123 Ω^-1 cm^-1 (at T
≈ 5 K) to the maximum value of ∼ 366 Ω^-1 cm^-1 near
T_SR. While the low-temperature part may originate due to the intrinsic KL
mechanism, our analysis indicates that the temperature-dependent AHC is
primarily appearing due to the side-jump mechanism as a result of the spin-flip
electron-magnon scattering. Our study demonstrates an interplay between
magnetism and band topology and its consequence on electron transport in
Fe_4GeTe_2.
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关键词
anomalous hall effect,unusual magnetotransport,quasi-two-dimensional
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