A non-centrosymmetric chalcohalide synthesized through the combination of chemical tailoring with aliovalent substitution.
Chemical communications (Cambridge, England)(2023)
摘要
A new non-centrosymmetric (NCS) chalcohalide, [SrCl][GeS], was successfully designed and synthesized through combining chemical tailoring with aliovalent substitution strategies from the maternal [NaSrCl][GeS]. It can exhibit a large SHG effect (0.97 × AgGaS), a wide band gap of 3.71 eV, and a high LDT (∼16 × AgGaS). These results indicate that [SrCl][GeS] may be a potential infrared nonlinear optical crystal.
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关键词
aliovalent substitution,chemical tailoring,non-centrosymmetric
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