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Rh(III)-catalyzed synthesis of amino-side-chained poly(phenylene vinylene) via C-H bond olefination.

Benfa Chu,Shuqi Jia,Tielei Li,Jin Zhu

Chemical communications (Cambridge, England)（2023）

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Abstract
A Rh(III)-catalyzed hydrazine-directed C-H olefination approach was developed for synthesizing amino-side-chained poly(phenylene vinylene) (PPV). The creation of such a divergent portfolio of PPV candidates enabled the discovery of a mega Stokes shift, high fluorescence quantum yield, and solid-state fluorescence, highlighting the great prospects of our synthetic protocol as an innovative tool.
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Key words
synthesis,rh<scp>iii</scp>-catalyzed,polyphenylene,amino-side-chained
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