Accessing Chiral Pyrrolodiketopiperazines under Organocatalytic Conditions
Organic Letters（2023）
Abstract
The production of chiral pyrrolodiketopiperazines under organocatalytic conditions demonstrates the capacity of bicyclic acylpyrrol lactims to perform as pronucleophiles in direct carbon–carbon bond forming reactions. The good performance of ureidoaminal-derived Brønsted bases in the Michael addition to nitroolefins affords these heterocyclic scaffolds with high skeleton diversity.
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Key words
chiral pyrrolodiketopiperazines,organocatalytic conditions
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