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Electronic, steric and catalytic properties of N-heterocyclic carbene rhodium(i) complexes linked to (metallo)porphyrins

Ludivine Poyac,Stefano Scoditti,Xavier Dumail,Michel Granier,Sebastien Clement,Rafael Gramage-Doria,Charles H. Devillers,Sebastien Richeter

CHEMICAL COMMUNICATIONS（2022）

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Abstract
Electronic and steric properties of NHC ligands functionalized with porphyrins were investigated. When porphyrins are used as NHC-wingtips, nickel(ii) in the macrocyle significantly improves the catalytic activity of the neighbouring NHC-Rh(i) complex in the conjugate addition of phenylboronic acid to cyclohexen-2-one.
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Key words
catalytic properties,complexes,rhodium<scp>i</scp>,n-heterocyclic
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