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Regulating Spin-State Switching by Integrating Polyoxometalate Anion into Spin Crossover System.

Jiajia Li,Xiao-Peng Sun, Shiqi Bi, Minglu Xu, Siyu Jia,Zheng Tang,Pengtao Ma,Jingping Wang,Jun Tao,Jingyang Niu

Inorganic chemistry（2022）

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Abstract
Polyoxometalate (POM) anions were successfully integrated into Fe(II) spin crossover (SCO) system, which demonstrates an effective role in regulating spin-state switching properties. Specifically, three drastically different magnetic behaviors of Fe(II) ion in the identical cation [Fe(bpp)] were achieved by leveraging [MoO], [MoO], and [Na(MoO)], respectively.
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Key words
integrating polyoxometalate anion,spin-state
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