Metal-to-metal electron transfer in a cyanido-bridged {Fe2Co2} square complex followed by X-ray diffraction and absorption techniques

Corine Mathonière,Dmitri Mitcov,Evangelia Koumousi, Daniel Amorin-Rosario,Pierre Dechambenoit,Sadaf Fatima Jafri,Philippe Sainctavit,Christophe Cartier Dit Moulin,Loic Toupet,Elzbieta Trzop,Eric Collet,Marie-Anne Arrio,Andrei Rogalev,Fabrice Wilhelm,Rodolphe Clérac

CHEMICAL COMMUNICATIONS（2022）

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摘要

The switching properties of a cyanido-bridged Fe/Co square molecule were investigated by single-crystal X-ray diffraction and X-ray absorption spectroscopy at both Fe and Co K-edges. Combining these two techniques, a complete picture of the thermal-, light- and X-ray-induced metal-to-metal electron transfer is obtained, illustrating the concerted role played by the Fe and Co sites.

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关键词

electron,transfer,metal-to-metal,cyanido-bridged,x-ray

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